Simple green for various exterior surfaces of a bike to degrease? Sure, just use it carefully,
remove fully when done cleaning with it, and avoid any areas where it can creep in where you can't thoroughly remove all of it (i.e. avoid all bearings and bushings).
But simple green for a chain? Not a good idea.
Why? Simple green is corrosive and it is thin enough that it can easily get inside the chain bushings. Simple green cuts oil and grease very very effectively and, once it is inside the chain, it will prevent chain lubricant from working like it should. And, depending on how much simple green gets inside the chain, it will/may begin corroding the inside of the chain. The best way (well, the fastest and cheapest way) to clean your chain is to just do it on your bike, in most cases, with the same lubricant you normally use for your chain plus an old rag.
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Advanced Aero TopTube Storage for Road, Gravel, & Tri...ZeroSlip & Direct-mount, made in the USA.
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